20 1001 Theresa Klausner (theresa.klausner(at)dlr.de), Anke Roiger (anke.roiger(at)dlr.de), Lisa Eirenschmalz (lisa.eirenschmalz(at)dlr.de), PI: Hans Schlager (hans.schlager(at)dlr.de) Deutsches Zentrum fuer Luft- und Raumfahrt, Institut fuer Physik der Atmosphaere, Oberpfaffenhofen, Germany 1 | HALO | CI-ITMS | Measurements of SO2 with Chemical Ionization Ion Trap Mass Spectrometry OMO 1 1 2015 07 28 2016 04 12 0 UTC (seconds after midnight) 1 1.0 99999 SO2 Mixing Ratio, (pptv) 4 OMO flight No. 10 OPERATOR on flight: Greta Stratmann Detection limit: 26 pptv No data after 10.30 UTC due to instrumental problems 1 UTC SO2 18445 99999 18456 99999 18468 99999 18479 99999 18490 99999 18500 99999 18510 99999 18521 99999 18531 99999 18541 99999 18551 99999 18561 99999 18571 99999 18580 99999 18590 99999 18601 99999 18611 99999 18621 99999 18631 99999 18642 99999 18652 99999 18662 99999 18672 99999 18682 99999 18692 99999 18703 99999 18713 99999 18723 99999 18733 99999 18743 99999 18753 99999 18763 99999 18773 99999 18783 99999 18794 99999 18804 99999 18814 99999 18824 99999 18834 99999 18844 99999 18854 99999 18864 99999 18874 99999 18884 99999 18894 99999 18906 99999 18922 99999 18938 99999 18954 99999 18971 99999 18987 99999 19003 99999 19020 99999 19036 99999 19052 99999 19068 99999 19085 99999 19101 99999 19117 99999 19134 99999 19150 99999 19166 99999 19183 99999 19199 99999 19215 99999 19231 99999 19248 99999 19264 99999 19280 99999 19297 99999 19313 99999 19329 99999 19346 99999 19362 99999 19378 99999 19394 99999 19411 99999 19426 99999 19442 99999 19458 99999 19475 99999 19491 99999 19507 99999 19524 99999 19540 99999 19556 99999 19572 99999 19588 99999 19605 99999 19621 99999 19637 99999 19653 99999 19670 99999 19686 99999 19702 99999 19718 99999 19734 99999 19750 99999 19766 99999 19782 99999 19799 99999 19815 99999 19831 99999 19847 99999 19863 99999 19880 99999 19896 99999 19912 99999 19928 99999 19944 99999 19961 99999 19977 99999 19993 99999 20009 99999 20025 99999 20041 99999 20057 99999 20074 99999 20090 99999 20106 99999 20122 99999 20139 99999 20155 99999 20171 99999 20188 99999 20204 99999 20220 99999 20237 99999 20253 99999 20270 99999 20286 99999 20303 99999 20319 99999 20335 99999 20352 99999 20368 99999 20384 99999 20400 99999 20417 99999 20433 99999 20449 99999 20465 99999 20481 99999 20497 99999 20514 99999 20530 99999 20546 99999 20562 99999 20578 99999 20595 99999 20611 99999 20627 99999 20643 99999 20660 99999 20676 99999 20692 99999 20708 99999 20724 99999 20741 99999 20757 99999 20773 99999 20790 99999 20806 99999 20823 99999 20840 99999 20857 99999 20874 99999 20888 99999 20900 99999 20912 99999 20924 99999 20936 99999 20948 99999 20959 99999 20970 99999 20981 99999 20992 99999 21003 99999 21014 99999 21024 99999 21035 99999 21045 99999 21056 99999 21066 99999 21077 99999 21088 99999 21098 99999 21108 99999 21119 99999 21130 99999 21140 99999 21150 99999 21161 99999 21171 99999 21182 99999 21192 99999 21202 99999 21213 99999 21223 99999 21233 99999 21244 99999 21254 99999 21264 99999 21275 99999 21285 99999 21296 99999 21306 99999 21317 99999 21327 99999 21338 99999 21348 99999 21358 99999 21369 99999 21379 99999 21389 99999 21400 99999 21410 99999 21421 99999 21431 99999 21442 99999 21452 99999 21462 99999 21473 99999 21483 99999 21493 99999 21504 99999 21514 99999 21525 99999 21535 99999 21545 99999 21555 99999 21566 99999 21576 99999 21587 99999 21597 99999 21608 99999 21618 99999 21629 99999 21639 99999 21650 99999 21660 99999 21671 99999 21682 99999 21693 99999 21704 99999 21715 99999 21726 99999 21738 99999 21748 99999 21759 99999 21770 99999 21781 99999 21791 99999 21802 99999 21813 99999 21824 99999 21835 99999 21845 99999 21856 99999 21867 99999 21877 99999 21888 99999 21899 99999 21909 99999 21920 99999 21930 99999 21940 99999 21951 99999 21961 99999 21971 99999 21982 99999 21992 99999 22003 99999 22014 99999 22025 99999 22036 99999 22046 99999 22057 99999 22067 99999 22078 99999 22089 99999 22100 99999 22110 99999 22120 99999 22131 99999 22141 99999 22151 99999 22162 99999 22172 99999 22183 99999 22193 99999 22203 99999 22213 99999 22223 99999 22234 99999 22244 99999 22254 99999 22264 99999 22275 99999 22285 99999 22295 99999 22305 99999 22315 99999 22325 99999 22335 99999 22345 99999 22356 99999 22366 99999 22376 99999 22386 99999 22397 99999 22407 99999 22418 99999 22428 99999 22439 99999 22449 99999 22460 99999 22470 99999 22479 99999 22489 99999 22499 99999 22510 99999 22520 99999 22530 99999 22540 99999 22549 99999 22559 99999 22569 99999 22579 99999 22589 99999 22599 99999 22610 24 22620 23 22631 23 22641 99999 22652 22 22662 16 22673 29 22684 20 22694 30 22705 53 22716 43 22727 64 22739 99999 22750 40 22762 99999 22773 29 22784 39 22794 99999 22804 16 22815 99999 22825 34 22835 18 22845 22 22856 99999 22866 23 22876 29 22887 30 22898 19 22908 38 22919 24 22930 40 22941 16 22952 42 22963 18 22974 31 22985 31 22996 43 23007 48 23018 28 23029 15 23040 34 23050 36 23061 37 23072 35 23083 50 23093 26 23104 38 23115 44 23125 31 23136 25 23146 29 23156 24 23167 18 23177 17 23187 26 23198 47 23208 29 23218 42 23228 21 23239 24 23249 99999 23259 20 23270 22 23280 38 23290 37 23300 32 23311 39 23321 30 23331 30 23342 25 23352 26 23362 23 23373 25 23384 37 23395 43 23405 30 23416 25 23426 45 23436 29 23446 18 23456 39 23465 39 23475 23 23484 99999 23494 36 23505 21 23515 40 23525 38 23535 20 23545 25 23555 14 23565 41 23575 29 23585 37 23594 32 23604 34 23615 28 23626 38 23636 43 23647 25 23657 24 23668 42 23679 21 23689 35 23700 21 23710 21 23721 29 23732 31 23743 24 23753 47 23764 28 23775 36 23785 54 23796 19 23807 39 23818 24 23828 38 23839 42 23850 42 23861 18 23871 23 23882 32 23893 29 23904 32 23915 36 23926 30 23937 27 23947 36 23958 25 23969 34 23980 31 23991 13 24002 99999 24013 31 24024 21 24035 22 24046 29 24057 9 24067 16 24078 17 24088 17 24099 21 24109 32 24120 20 24130 10 24141 23 24151 19 24162 99999 24173 30 24183 23 24194 39 24204 14 24215 18 24225 19 24236 16 24246 26 24256 33 24267 13 24277 10 24288 20 24298 22 24308 12 24319 20 24329 15 24339 29 24350 11 24360 19 24370 28 24381 15 24391 99999 24401 38 24411 11 24422 11 24432 18 24442 14 24452 11 24462 10 24472 26 24483 13 24493 34 24504 32 24514 28 24525 29 24536 27 24546 99999 24557 15 24568 99999 24579 99999 24589 8 24600 23 24610 31 24621 99999 24631 21 24642 99999 24652 21 24663 18 24674 15 24684 19 24695 13 24705 6 24715 28 24726 23 24736 15 24747 13 24757 30 24768 24 24779 11 24790 14 24801 99999 24811 14 24822 24 24833 99999 24844 12 24855 10 24866 29 24878 8 24889 99999 24900 19 24911 18 24922 99999 24933 18 24943 99999 24954 18 24965 26 24976 24 24986 15 24997 23 25008 32 25019 99999 25030 99999 25041 28 25052 99999 25063 15 25074 34 25084 28 25095 11 25105 23 25116 99999 25126 18 25137 20 25148 33 25159 99999 25170 13 25181 22 25192 99999 25203 10 25214 29 25225 99999 25236 99999 25247 14 25258 27 25269 9 25281 34 25292 26 25303 17 25314 19 25325 12 25335 13 25346 99999 25357 15 25368 99999 25379 14 25390 23 25401 99999 25412 33 25423 22 25434 15 25445 27 25456 21 25467 26 25477 19 25488 21 25499 15 25510 20 25520 21 25531 13 25542 10 25553 15 25563 23 25574 38 25585 99999 25605 17 25616 15 25627 27 25638 18 25649 19 25659 26 25670 16 25681 48 25692 21 25703 17 25713 17 25724 16 25735 20 25746 12 25756 26 25767 18 25778 11 25788 28 25799 30 25809 20 25819 99999 25830 27 25840 14 25851 99999 25861 13 25871 14 25882 16 25892 11 25902 13 25912 21 25923 8 25933 26 25943 37 25953 21 25963 15 25974 25 25984 99999 25994 10 26004 10 26014 99999 26024 99999 26034 28 26045 99999 26055 20 26065 13 26075 10 26085 6 26095 27 26105 36 26115 99999 26125 19 26135 25 26146 29 26156 27 26166 20 26176 7 26187 14 26197 7 26207 17 26218 22 26228 45 26239 10 26249 19 26260 25 26271 25 26281 25 26292 29 26303 22 26314 23 26324 25 26335 15 26346 27 26356 27 26367 16 26377 21 26388 14 26398 18 26409 20 26419 22 26430 16 26441 17 26451 22 26462 23 26473 99999 26484 99999 26494 22 26505 15 26515 22 26526 16 26536 29 26547 99999 26558 20 26569 9 26579 30 26590 28 26600 24 26611 30 26621 19 26632 14 26643 26 26653 99999 26664 13 26675 35 26685 28 26696 11 26706 14 26717 15 26727 14 26737 99999 26748 26 26759 21 26770 23 26780 12 26791 28 26802 20 26813 20 26824 19 26835 99999 26845 22 26856 23 26866 21 26877 14 26887 27 26898 99999 26909 27 26919 25 26930 30 26941 37 26952 24 26962 24 26973 23 26984 29 26995 14 27006 19 27017 9 27027 19 27038 12 27049 21 27060 17 27071 99999 27081 11 27092 16 27103 28 27114 28 27124 35 27135 29 27146 38 27156 22 27167 30 27178 21 27189 24 27199 36 27210 25 27220 34 27231 19 27242 17 27252 26 27263 31 27274 20 27284 22 27295 32 27305 21 27316 38 27327 17 27337 33 27347 25 27358 27 27368 30 27378 33 27389 35 27399 28 27410 17 27420 17 27429 26 27439 14 27449 99999 27459 31 27469 16 27479 18 27489 23 27499 24 27510 21 27519 24 27529 26 27539 18 27548 22 27558 32 27568 23 27578 23 27588 26 27598 12 27608 33 27618 14 27627 20 27637 40 27647 25 27657 19 27666 16 27676 25 27686 16 27696 34 27706 20 27716 22 27726 30 27736 21 27746 25 27756 29 27767 33 27777 19 27787 25 27797 24 27807 11 27817 26 27827 12 27837 24 27847 13 27856 17 27866 26 27876 28 27886 6 27895 25 27905 25 27915 24 27925 23 27935 15 27945 18 27955 33 27964 20 27974 5 27984 17 27993 99999 28003 16 28012 22 28022 13 28032 27 28042 7 28052 24 28062 22 28071 25 28081 32 28091 18 28101 21 28110 41 28120 13 28130 35 28140 17 28150 22 28160 27 28178 22 28187 17 28197 7 28207 15 28216 99999 28226 20 28236 15 28246 17 28256 35 28266 22 28277 18 28288 23 28299 51 28310 31 28321 43 28331 17 28338 27 28346 21 28354 9 28362 33 28370 25 28378 47 28385 30 28393 27 28402 21 28410 27 28418 17 28426 18 28434 15 28442 19 28450 14 28458 20 28467 20 28475 26 28483 16 28491 18 28499 19 28508 10 28516 12 28524 6 28532 25 28540 21 28549 99999 28557 16 28566 17 28574 23 28583 99999 28592 25 28600 16 28609 20 28617 14 28626 15 28635 19 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36 31387 17 31395 29 31404 31 31412 19 31421 28 31429 40 31438 33 31446 37 31455 28 31463 30 31472 35 31480 38 31489 33 31497 43 31506 25 31514 35 31522 24 31531 31 31539 23 31548 24 31556 33 31564 24 31572 30 31581 27 31589 31 31597 32 31606 29 31614 30 31622 25 31630 37 31639 37 31647 28 31655 27 31664 38 31672 28 31680 19 31689 26 31697 31 31706 26 31714 35 31722 26 31731 18 31739 31 31748 31 31756 23 31764 32 31773 31 31781 28 31789 24 31798 27 31806 33 31814 48 31822 41 31830 32 31838 44 31846 49 31854 44 31864 44 31877 38 31885 39 31893 36 31901 36 31909 36 31917 26 31926 31 31934 32 31942 24 31950 29 31958 18 31967 20 31975 21 31983 31 31991 31 31999 31 32007 29 32015 32 32024 33 32032 27 32040 35 32048 37 32056 31 32064 20 32073 16 32081 21 32090 12 32098 6 32106 13 32114 12 32123 15 32131 16 32139 20 32146 17 32154 99999 32162 16 32170 10 32178 15 32186 18 32194 11 32202 17 32210 15 32218 10 32225 26 32233 16 32241 11 32249 24 32257 20 32264 20 32272 99999 32280 9 32288 9 32295 16 32303 7 32311 11 32319 12 32326 14 32334 18 32342 10 32350 14 32357 11 32365 9 32373 17 32380 17 32388 15 32396 99999 32404 12 32412 15 32419 99999 32427 9 32435 10 32442 17 32450 18 32458 13 32466 99999 32474 14 32481 22 32489 11 32497 13 32505 12 32512 16 32520 11 32528 19 32536 99999 32544 9 32551 15 32559 23 32567 14 32575 12 32583 13 32590 16 32598 7 32606 16 32614 4 32622 8 32629 13 32637 7 32645 15 32653 99999 32661 99999 32669 14 32676 8 32684 9 32692 11 32701 26 32709 27 32717 18 32725 21 32734 25 32742 20 32751 26 32759 30 32767 23 32776 18 32785 15 32793 46 32802 53 32811 33 32819 16 32828 13 32837 18 32846 26 32855 12 32865 26 32874 24 32883 24 32891 15 32900 29 32909 20 32918 20 32926 20 32935 99999 32944 22 32952 17 32961 16 32970 20 32978 24 32987 16 32995 20 33004 17 33013 32 33021 23 33030 22 33038 37 33047 29 33056 18 33064 26 33073 27 33081 19 33090 30 33099 14 33108 15 33117 20 33126 15 33135 20 33144 16 33153 20 33162 12 33170 15 33179 21 33188 11 33198 8 33207 24 33216 22 33225 20 33234 11 33243 14 33252 16 33261 25 33270 99999 33279 8 33288 12 33297 15 33306 22 33315 99999 33324 17 33334 24 33343 9 33352 10 33361 99999 33370 99999 33379 17 33388 99999 33398 14 33407 15 33416 17 33425 99999 33434 12 33444 10 33453 15 33462 12 33472 99999 33481 99999 33491 31 33500 10 33510 14 33519 8 33528 21 33537 17 33547 11 33556 7 33565 15 33574 7 33584 14 33593 13 33602 16 33611 11 33620 12 33629 99999 33639 10 33648 21 33657 13 33666 27 33675 14 33684 14 33693 12 33703 8 33712 22 33721 16 33730 30 33739 40 33748 14 33758 14 33767 7 33776 10 33785 7 33794 99999 33803 12 33812 10 33821 12 33831 12 33840 15 33849 11 33858 21 33867 16 33876 23 33885 9 33894 18 33903 14 33912 13 33921 15 33930 14 33939 11 33948 9 33957 16 33967 14 33976 8 33985 14 33993 13 34002 99999 34012 14 34021 99999 34029 23 34038 99999 34047 16 34056 18 34065 19 34074 99999 34083 99999 34092 15 34102 11 34111 99999 34120 99999 34129 99999 34139 99999 34148 99999 34158 99999 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36037 21 36046 23 36055 14 36063 12 36072 21 36081 16 36090 18 36098 18 36107 15 36116 16 36124 14 36133 14 36142 26 36150 17 36159 19 36168 20 36176 29 36185 20 36193 13 36202 27 36211 17 36219 20 36228 26 36236 33 36245 29 36253 35 36262 19 36270 22 36279 28 36287 20 36296 19 36305 26 36313 37 36322 38 36330 20 36339 27 36347 17 36356 13 36364 20 36373 29 36381 31 36390 34 36398 28 36407 21 36415 40 36424 33 36433 24 36441 20 36450 17 36458 24 36467 22 36476 25 36484 23 36493 30 36502 47 36511 23 36519 29 36528 25 36537 30 36545 19 36554 33 36563 24 36571 18 36580 24 36589 16 36598 15 36607 23 36616 9 36625 13 36634 18 36643 11 36652 99999 36662 99999 36671 20 36680 10 36689 15 36698 8 36707 99999 36716 26 36725 16 36734 14 36743 9 36752 10 36761 10 36770 18 36779 15 36789 8 36798 7 36807 99999 36816 17 36826 9 36835 13 36844 99999 36853 19 36863 11 36872 19 36881 9 36891 18 36900 99999 36909 15 36918 24 36928 7 36937 8 36946 8 36956 22 36965 99999 36974 18 36983 99999 36992 16 37002 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