72 1001 Markus Jesswein, Thomas Wagenhaeuser, Timo Keber, Tanja Schuck, Andreas Engel Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhoeferallee 1, 60438 Frankfurt/Main, Germany 1 | HALO | GhOST-MS | mixing ratios of long-lived and very short-lived tracers measured with an in-situ GC-MS instrument SOUTHTRAC 1 1 2019 09 18 2020 08 24 0 Mean sample time in UT seconds past midnight of flight date 25 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 C2Cl4 [ppt] C2H3Cl3 [ppt] CCl4 [ppt] CFC11 [ppt] CFC113 [ppt] CFC114 [ppt] CFC115 [ppt] CFC12 [ppt] CH2Br2 [ppt] CH2Cl2 [ppt] CH3Br [ppt] CH3Cl [ppt] CH3I [ppt] CHBr2Cl [ppt] CHBr3 [ppt] CHCl3 [ppt] H1211 [ppt] H1301 [ppt] H2402 [ppt] HCFC141b [ppt] HCFC142b [ppt] HCFC22 [ppt] HFC125 [ppt] HFC134a [s] HFC143a [s] 31 ------------------------------------------------------------------------ Please inform the authors about the use of the data Before publication, the authors of the data have to give their consent Please adhere in all cases to the SOUTHTRAC data protocol Contact: Andreas Engel (an.engel@iau.uni-frankfurt.de, phone +49 69 798 40259) ------------------------------------------------------------------------ Calibration Scale, Precision, Accuracy and Detection Limit are given separately for each dependent variable Primary calibration reference flasks: AGAGE H-218 (all other scales) Calibration Scales NOAA-2003B SIO-05 SIO-05 SIO-05 SIO-05 SIO-05 SIO-05 SIO-05 NOAA-2003 SIO-14 SIO-05 SIO-05 NOAA-2004 UEA-11 NOAA-2003 SIO-05 SIO-05 SIO-05 SIO-14 SIO-05 SIO-05 SIO-05 SIO-14 SIO-05 SIO-07 ------------------------------------------------------------------------ Instrument precision in [%] 0.0131 0.0867 0.0044 0.0022 0.0064 0.0073 0.0140 0.0030 0.0259 0.0078 0.0169 0.0039 0.0675 0.0891 0.0282 0.0095 0.0278 0.0383 0.0579 0.0082 0.0084 0.0041 0.0079 0.0049 0.0167 Instrument precision in [ppt] 0.0800 0.1527 0.3524 0.5192 0.4049 0.1199 0.1238 1.5384 0.0330 0.5550 0.1154 2.7873 0.0186 0.0677 0.0492 0.1397 0.0929 0.1349 0.0226 0.2095 0.1932 1.0807 0.3451 1.7285 0.43155 Use whatever precision is larger for each data point ------------------------------------------------------------------------ Accuracy of mixing ratios in calibration gas in [%] NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN ------------------------------------------------------------------------ Detection limit (S/N 3/1) in [ppt] per 400 mL air at STP 0.11162 0.53190 0.19529 0.35685 0.18416 0.11912 0.32568 0.47153 0.11040 0.45926 0.30992 3.50523 0.07732 0.74990 0.24115 0.65568 0.25124 0.93355 0.08583 0.39324 0.4981 1.30346 0.625 0.76391 1.86463 Values below detection limit are marked as 0.00 In case no measurements are available, the missing data value is used ------------------------------------------------------------------------ Sample integration time: 147 +- 1 seconds Values of t_sample are the mean of the sampling time interval (integration time) ------------------------------------------------------------------------ Correction of analyte carry-over (memory effect): below measurement precision for all substances, no correction applied Detector non-linearity: below measurement precision for all substances, no correction applied ------------------------------------------------------------------------ 2 TIME C2Cl4 C2H3Cl3 CCl4 CFC11 CFC113 CFC114 CFC115 CFC12 CH2Br2 CH2Cl2 CH3Br CH3Cl CH3I CHBr2Cl CHBr3 CHCl3 H1211 H1301 H2402 HCFC141b HCFC142b HCFC22 HFC125 HFC134a HFC143a [s] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [s] [s] 82898.0 1.381 5.132 77.299 231.650 99999.000 15.557 8.848 502.583 1.152 26.191 16.303 703.148 0.652 2.603 2.455 14.712 4.648 3.598 0.000 22.283 21.793 233.731 28.913 100.009 0.000 83606.0 0.579 1.100 79.643 228.569 99999.000 15.452 9.094 510.816 1.217 19.285 5.875 541.100 0.198 0.553 1.034 7.295 3.209 3.583 0.000 23.477 22.101 239.770 28.887 99.476 0.000 83959.0 0.436 1.028 75.235 219.732 69.335 15.653 9.050 507.604 0.801 21.489 6.998 555.144 0.065 0.239 0.400 5.763 3.659 3.621 0.000 23.016 22.023 239.054 27.498 100.425 0.000 84313.0 0.165 1.057 71.061 215.948 68.215 15.793 9.219 512.943 0.578 22.706 7.133 576.911 0.060 99999.000 0.128 4.346 3.060 3.480 0.000 22.760 23.209 257.052 29.345 101.581 0.000 84667.0 99999.000 0.824 62.250 187.133 63.088 15.250 9.148 476.000 0.391 18.418 6.240 496.128 0.067 99999.000 0.037 3.376 2.556 3.287 0.000 20.910 21.881 240.251 25.608 94.391 0.000 85021.0 0.068 0.887 57.456 177.150 61.043 14.763 8.249 442.276 0.323 17.719 5.879 456.644 0.059 99999.000 99999.000 3.184 2.358 2.727 0.000 20.414 21.318 220.844 23.684 91.248 0.000 85375.0 0.065 0.970 58.363 186.050 61.271 14.672 8.296 440.818 0.336 17.758 5.831 450.479 0.050 99999.000 99999.000 3.455 2.437 3.042 0.000 20.674 20.836 218.594 23.592 90.765 0.000 85728.0 0.056 0.947 61.372 190.767 63.561 14.767 8.491 455.977 0.366 19.019 6.057 483.751 0.088 99999.000 99999.000 3.323 2.612 3.011 0.000 21.132 21.236 226.341 24.966 93.421 0.000 86082.0 0.057 0.904 61.082 192.405 62.659 14.825 8.328 451.186 0.349 18.462 6.007 464.471 0.060 99999.000 99999.000 3.241 2.556 2.941 0.000 20.836 20.803 225.814 24.196 91.530 0.000 86435.0 99999.000 0.916 57.403 181.817 60.763 14.687 8.475 441.027 0.339 17.471 5.772 444.318 0.066 99999.000 99999.000 3.336 2.407 2.694 0.000 20.294 20.570 222.998 23.545 89.906 0.000 87140.0 0.074 0.920 57.633 171.727 99999.000 14.447 8.240 435.553 0.339 17.766 5.790 436.596 0.060 99999.000 99999.000 3.304 2.431 2.873 0.000 20.566 20.389 217.341 23.402 88.244 0.000 87494.0 99999.000 0.868 57.775 188.992 61.388 14.901 8.469 447.399 0.346 17.930 5.784 462.723 0.062 99999.000 99999.000 3.159 2.421 2.665 0.000 20.397 20.896 227.804 24.498 91.465 0.000 87846.0 99999.000 0.992 57.416 187.493 60.913 14.556 8.326 438.839 0.355 17.736 5.711 439.300 0.065 99999.000 99999.000 2.967 2.431 2.833 0.000 20.259 20.329 221.244 23.797 88.683 0.000 88200.0 99999.000 0.825 54.080 178.075 59.672 14.622 8.125 422.055 0.304 16.406 5.486 426.453 0.074 99999.000 0.035 3.017 2.235 2.847 0.000 19.232 20.128 213.877 23.240 88.648 0.000 88553.0 99999.000 0.749 50.150 157.941 57.429 14.169 8.272 415.651 0.270 14.936 4.788 406.994 0.078 99999.000 99999.000 2.622 2.194 2.756 0.000 18.661 19.930 216.500 22.555 86.621 0.000 88906.0 99999.000 0.971 51.558 158.406 57.826 14.369 8.544 421.296 0.274 15.528 5.163 420.436 0.084 99999.000 99999.000 2.635 2.126 2.650 0.000 18.699 20.062 215.664 22.671 88.074 0.000 89259.0 99999.000 0.840 49.152 162.458 56.376 14.393 8.494 412.885 0.250 15.038 4.865 405.607 0.081 99999.000 99999.000 2.446 2.030 2.736 0.000 18.312 20.080 218.586 22.637 86.213 0.000 89612.0 0.068 0.845 49.496 153.306 56.897 14.246 8.522 415.506 0.245 14.740 4.854 403.089 0.086 99999.000 99999.000 2.666 2.047 2.511 0.000 18.661 20.340 216.731 23.131 85.769 0.000 89966.0 0.047 0.810 51.380 164.774 58.046 14.397 8.706 422.466 0.280 15.321 5.082 418.933 0.058 99999.000 99999.000 2.748 2.141 2.770 0.000 18.937 20.413 219.167 23.449 87.981 0.000 90673.0 0.073 0.926 57.397 175.496 99999.000 14.613 8.632 443.674 0.355 17.914 5.713 454.628 0.057 99999.000 99999.000 3.024 2.542 2.813 0.000 20.277 20.865 224.207 24.684 91.186 0.000 91027.0 99999.000 0.990 58.603 181.504 61.638 14.889 8.514 440.440 0.359 17.952 5.617 463.763 0.087 99999.000 99999.000 3.035 2.476 2.903 0.000 20.457 20.886 223.054 23.689 90.837 0.000 91380.0 0.069 1.007 61.818 199.210 62.989 15.160 8.620 457.964 0.385 19.298 5.791 475.185 0.093 99999.000 99999.000 3.204 2.646 3.104 0.000 20.789 21.378 233.162 25.131 93.398 0.000 91733.0 0.059 0.965 59.225 177.214 62.158 14.839 8.446 448.358 0.359 17.818 5.634 460.350 0.078 99999.000 99999.000 3.090 2.451 2.794 0.000 20.689 20.521 225.740 23.988 91.270 0.000 92086.0 0.063 0.876 58.285 177.616 61.231 14.618 8.368 440.473 0.321 17.463 5.612 453.540 0.085 99999.000 99999.000 3.102 2.423 2.816 0.000 20.350 21.042 221.962 24.590 89.831 0.000 92440.0 0.048 0.863 56.053 171.313 60.696 14.729 8.469 441.349 0.323 16.917 5.540 448.585 0.093 99999.000 99999.000 2.877 2.369 2.840 0.000 19.825 20.728 226.528 24.498 89.697 0.000 92794.0 99999.000 0.979 59.508 178.921 62.271 15.019 8.629 455.459 0.353 18.565 5.727 475.224 0.096 99999.000 99999.000 3.469 2.532 2.804 0.000 20.563 20.812 231.676 25.085 91.863 0.000 93147.0 99999.000 0.930 63.304 198.058 64.067 15.080 8.434 471.573 0.408 20.323 6.456 506.472 0.096 99999.000 99999.000 3.483 2.679 3.021 0.000 21.391 21.241 236.799 25.671 94.405 0.000 93501.0 0.248 1.071 73.753 227.979 69.526 15.916 8.750 501.287 0.633 33.879 6.974 570.346 0.070 99999.000 0.094 5.416 3.299 3.231 0.000 23.895 21.873 248.970 28.770 102.393 0.000 94207.0 0.134 1.078 65.498 195.439 99999.000 15.165 8.459 462.597 0.445 23.130 6.344 496.412 0.075 99999.000 99999.000 3.714 2.817 2.939 0.000 21.563 21.349 228.094 25.859 94.965 0.000 94561.0 0.117 0.929 63.984 193.852 64.356 15.088 8.390 460.735 0.421 22.431 6.578 496.931 0.076 99999.000 99999.000 3.821 2.715 3.185 0.000 21.381 21.109 222.889 25.122 92.811 0.000 94914.0 0.104 0.944 62.653 189.633 63.744 15.176 8.254 455.478 0.393 20.334 6.403 486.834 0.069 99999.000 99999.000 3.378 2.710 2.938 0.000 21.217 21.015 228.055 25.359 93.659 0.000 95267.0 99999.000 0.909 58.866 191.083 61.392 15.057 8.330 447.893 0.358 18.146 5.807 462.557 0.084 99999.000 99999.000 3.084 2.531 2.740 0.000 20.523 20.921 226.467 24.095 90.576 0.000 95620.0 0.075 0.941 62.223 188.096 63.780 14.932 8.244 450.643 0.363 18.994 6.250 481.596 0.082 99999.000 99999.000 3.493 2.640 2.974 0.000 21.168 21.361 224.043 25.306 92.577 0.000 95974.0 0.043 0.925 58.668 180.765 61.698 14.783 8.115 446.118 0.316 17.943 6.033 464.201 0.080 99999.000 99999.000 3.178 2.493 2.780 0.000 20.312 20.433 224.125 23.689 90.925 0.000 96328.0 0.105 0.982 65.260 188.977 65.013 14.922 8.236 464.509 0.427 22.183 6.519 500.032 0.086 99999.000 99999.000 4.123 2.790 3.058 0.000 21.792 20.817 237.416 26.045 94.226 0.000 96682.0 0.146 1.008 68.483 200.166 66.893 15.123 8.353 480.476 0.472 24.538 7.241 531.922 0.075 99999.000 99999.000 4.106 2.939 3.187 0.000 22.502 21.232 236.561 27.658 97.175 0.000 97035.0 99999.000 0.952 59.184 189.982 62.002 14.947 8.134 448.473 0.341 18.742 6.219 468.731 0.099 99999.000 99999.000 3.316 2.471 2.882 0.000 20.544 20.741 229.304 25.324 91.190 0.000 97740.0 0.258 1.144 76.555 226.250 99999.000 15.674 8.274 498.516 0.666 35.565 7.553 584.569 99999.000 99999.000 0.098 5.862 3.367 3.592 0.000 24.098 21.996 242.686 28.935 102.071 0.000 98093.0 0.219 0.995 75.074 232.856 70.000 15.917 8.502 497.258 0.598 33.883 7.384 571.967 0.042 99999.000 0.083 5.452 3.217 3.477 0.000 23.687 22.026 240.549 28.364 102.824 0.000 98447.0 0.256 1.080 76.483 223.996 70.587 15.601 8.449 503.750 0.666 37.421 7.642 589.221 0.067 99999.000 0.106 5.780 3.282 3.578 0.000 24.023 22.300 250.601 29.718 103.973 0.000 98801.0 0.153 0.999 73.262 216.975 69.044 15.472 8.503 495.195 0.546 30.768 7.221 562.794 0.057 99999.000 0.065 5.218 3.074 3.350 0.000 23.285 21.843 243.624 29.160 100.423 0.000 99154.0 99999.000 1.003 73.266 215.426 69.185 15.396 8.469 492.650 0.565 30.403 7.402 561.778 0.073 99999.000 0.044 4.971 3.077 3.419 0.000 23.429 22.063 241.763 28.112 99.926 0.000 99506.0 0.185 1.083 73.574 216.225 70.051 15.575 8.431 495.742 0.610 34.311 7.445 562.896 0.055 99999.000 0.075 5.307 3.075 3.487 0.000 23.626 22.338 243.389 28.723 101.006 0.000 99859.0 0.153 1.135 75.168 215.422 69.821 15.758 8.608 494.278 0.589 33.096 7.376 560.815 0.054 99999.000 0.084 5.679 3.073 3.513 0.000 23.596 21.816 239.339 28.325 101.501 0.000 100212.0 0.059 0.905 58.872 193.492 63.285 14.923 8.479 453.328 0.349 18.843 6.076 476.055 0.071 99999.000 99999.000 3.128 2.449 2.858 0.000 21.069 20.771 226.259 25.229 92.196 0.000 100565.0 0.085 0.912 64.198 196.430 65.163 15.166 8.537 467.471 0.418 23.566 6.501 511.338 0.094 99999.000 99999.000 3.946 2.593 3.205 0.000 21.994 21.163 232.519 26.238 96.461 0.000 101271.0 0.061 0.810 54.787 173.520 99999.000 14.959 8.439 446.947 0.299 17.447 5.758 473.070 0.096 99999.000 99999.000 2.794 2.326 2.801 0.000 20.263 21.294 231.906 25.429 92.679 0.000 101624.0 99999.000 0.790 43.345 142.705 54.302 14.081 8.114 397.295 0.190 13.076 4.684 391.101 0.102 99999.000 99999.000 2.129 1.859 2.180 0.000 17.779 19.999 205.875 22.015 84.034 0.000 101977.0 99999.000 0.724 40.943 134.886 53.455 13.864 8.191 392.259 0.179 12.397 4.543 374.770 0.112 99999.000 99999.000 2.050 1.673 2.232 0.000 17.279 19.647 209.760 21.532 82.426 0.000 102330.0 99999.000 0.784 42.925 138.720 54.354 99999.000 8.459 393.957 0.176 12.888 4.500 378.836 0.084 99999.000 99999.000 2.196 1.717 2.500 0.000 17.971 19.835 206.027 21.505 82.743 0.000 102683.0 99999.000 0.810 44.783 151.194 54.924 14.376 8.058 402.113 0.220 12.908 4.948 399.417 0.099 99999.000 99999.000 2.325 1.820 2.403 0.000 17.964 19.991 210.757 22.398 84.869 0.000 103036.0 99999.000 0.893 53.649 167.824 60.289 14.623 8.146 427.630 0.290 16.381 5.693 444.103 0.094 99999.000 99999.000 2.732 2.245 2.441 0.000 19.583 20.337 219.714 23.434 88.453 0.000 103389.0 99999.000 0.669 40.589 138.351 52.586 13.761 7.994 382.929 0.184 11.916 4.348 363.722 0.113 99999.000 99999.000 1.989 1.604 1.942 0.000 16.916 19.292 203.209 20.729 80.574 0.000 103743.0 99999.000 0.561 29.227 106.730 45.492 13.228 7.826 342.010 0.119 8.979 3.468 306.645 0.105 99999.000 99999.000 1.440 1.377 1.615 0.000 14.630 18.802 196.620 19.950 75.915 0.000 104097.0 99999.000 0.571 28.044 99.990 44.769 13.063 7.791 336.998 0.089 8.364 3.295 299.445 0.107 99999.000 99999.000 1.391 1.369 1.387 0.000 14.116 18.588 192.167 19.426 74.801 0.000 104801.0 99999.000 0.697 38.186 130.460 99999.000 13.701 7.891 376.219 0.162 11.539 4.100 349.733 0.081 99999.000 99999.000 1.626 1.595 1.912 0.000 16.482 19.386 203.946 20.756 81.009 0.000 105155.0 99999.000 0.662 39.274 130.958 52.032 13.626 8.197 380.967 0.174 11.744 4.208 359.882 0.125 99999.000 99999.000 2.005 1.665 1.950 0.000 16.771 19.771 205.282 21.594 81.724 0.000 105508.0 99999.000 0.661 39.405 137.670 51.596 14.010 7.859 381.574 0.175 11.441 4.198 363.334 0.092 99999.000 99999.000 1.841 1.796 2.017 0.000 16.752 19.555 207.785 21.210 81.115 0.000 105862.0 0.026 0.694 41.207 142.597 52.664 13.770 8.105 387.467 0.175 12.427 4.436 374.913 0.098 99999.000 99999.000 2.109 1.858 2.256 0.000 17.116 19.939 205.993 21.090 83.220 0.000 106215.0 99999.000 0.707 41.868 135.504 52.741 99999.000 7.868 389.079 0.205 12.237 4.377 368.313 0.102 99999.000 99999.000 2.468 1.729 2.102 0.000 17.028 19.728 205.062 20.896 82.360 0.000 106569.0 99999.000 0.839 46.894 149.637 56.317 14.087 8.096 407.824 0.228 13.987 4.914 403.274 0.104 99999.000 99999.000 2.526 1.997 2.097 0.000 17.881 20.512 211.020 22.311 86.353 0.000 106922.0 99999.000 0.744 48.134 153.232 57.215 14.062 8.030 414.560 0.241 14.514 4.953 405.949 0.111 99999.000 99999.000 2.511 2.027 2.209 0.000 18.541 20.676 210.371 22.172 86.248 0.000 107276.0 99999.000 0.756 40.151 130.261 52.478 13.475 7.950 383.172 0.182 11.521 4.440 361.445 0.098 99999.000 99999.000 1.926 1.705 2.145 0.000 16.969 20.204 202.267 20.805 81.442 0.000 107629.0 99999.000 0.673 38.869 134.139 52.281 13.857 7.839 381.987 0.129 11.768 4.380 365.348 0.103 99999.000 99999.000 1.729 1.571 2.145 0.000 16.767 19.767 204.096 21.187 80.510 0.000 108333.0 0.041 0.815 48.528 156.325 99999.000 13.886 8.172 412.264 0.238 14.577 4.842 400.287 0.104 99999.000 99999.000 2.394 2.063 2.489 0.000 18.566 20.246 214.779 21.877 85.267 0.000 108686.0 99999.000 0.968 62.365 189.339 63.699 14.474 8.687 458.292 0.384 18.765 5.873 471.960 0.087 99999.000 99999.000 3.418 2.740 3.134 0.000 21.168 21.219 228.080 25.090 91.682 0.000 109076.0 0.061 0.989 68.499 202.832 66.666 15.002 8.651 484.696 0.488 21.019 6.878 527.766 0.092 99999.000 0.069 3.897 3.028 3.153 0.000 22.492 21.820 238.053 27.222 97.979 0.000 109466.0 0.190 0.991 72.993 211.343 69.858 14.962 8.960 492.144 0.662 22.358 7.098 547.594 0.075 99999.000 0.165 4.670 3.257 3.325 0.000 23.359 22.057 236.270 27.252 99.263 0.000 109819.0 0.457 1.259 77.432 223.756 70.921 15.450 8.763 503.566 1.012 21.161 6.532 572.435 0.120 0.247 0.641 6.526 3.395 3.523 0.000 24.020 22.128 238.467 28.932 102.043 0.000 110172.0 0.509 1.155 77.620 222.332 71.242 15.343 9.099 503.736 1.036 21.237 6.268 562.512 0.130 0.276 0.790 6.729 3.478 3.663 0.000 24.211 22.013 237.635 28.337 101.965 0.000 110525.0 99999.000 1.160 78.707 225.216 70.565 15.731 8.606 508.036 1.013 21.159 6.212 551.217 0.116 0.266 0.779 6.731 3.363 3.541 0.000 24.016 22.107 239.065 28.038 101.428 0.000 110878.0 99999.000 1.218 77.969 219.982 70.409 15.538 8.553 505.043 0.988 20.084 6.506 549.691 0.144 0.265 0.841 6.666 3.442 3.364 0.000 23.790 22.272 239.488 27.429 101.841 0.000 111231.0 0.539 1.197 78.190 234.194 69.972 15.515 8.790 501.750 0.997 20.516 6.232 542.984 0.167 0.331 1.033 6.683 3.328 3.401 0.000 23.703 21.751 237.891 27.843 99.365 0.000 111938.0 0.498 1.008 78.476 230.755 99999.000 15.804 8.585 500.943 1.020 19.776 5.675 528.596 0.227 0.418 1.534 10.516 3.331 3.461 0.000 24.366 21.923 234.368 27.898 99.597 0.000