72 1001 Markus Jesswein, Thomas Wagenhaeuser, Timo Keber, Tanja Schuck, Andreas Engel Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Altenhoeferallee 1, 60438 Frankfurt/Main, Germany 1 | HALO | GhOST-MS | mixing ratios of long-lived and very short-lived tracers measured with an in-situ GC-MS instrument SOUTHTRAC 1 1 2019 09 11 2020 08 24 0 Mean sample time in UT seconds past midnight of flight date 25 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 1 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 99999 C2Cl4 [ppt] C2H3Cl3 [ppt] CCl4 [ppt] CFC11 [ppt] CFC113 [ppt] CFC114 [ppt] CFC115 [ppt] CFC12 [ppt] CH2Br2 [ppt] CH2Cl2 [ppt] CH3Br [ppt] CH3Cl [ppt] CH3I [ppt] CHBr2Cl [ppt] CHBr3 [ppt] CHCl3 [ppt] H1211 [ppt] H1301 [ppt] H2402 [ppt] HCFC141b [ppt] HCFC142b [ppt] HCFC22 [ppt] HFC125 [ppt] HFC134a [s] HFC143a [s] 31 ------------------------------------------------------------------------ Please inform the authors about the use of the data Before publication, the authors of the data have to give their consent Please adhere in all cases to the SOUTHTRAC data protocol Contact: Andreas Engel (an.engel@iau.uni-frankfurt.de, phone +49 69 798 40259) ------------------------------------------------------------------------ Calibration Scale, Precision, Accuracy and Detection Limit are given separately for each dependent variable Primary calibration reference flasks: AGAGE H-218 (all other scales) Calibration Scales NOAA-2003B SIO-05 SIO-05 SIO-05 SIO-05 SIO-05 SIO-05 SIO-05 NOAA-2003 SIO-14 SIO-05 SIO-05 NOAA-2004 UEA-11 NOAA-2003 SIO-05 SIO-05 SIO-05 SIO-14 SIO-05 SIO-05 SIO-05 SIO-14 SIO-05 SIO-07 ------------------------------------------------------------------------ Instrument precision in [%] 0.0131 0.0867 0.0044 0.0022 0.0064 0.0073 0.0140 0.0030 0.0259 0.0078 0.0169 0.0039 0.0675 0.0891 0.0282 0.0095 0.0278 0.0383 0.0579 0.0082 0.0084 0.0041 0.0079 0.0049 0.0167 Instrument precision in [ppt] 0.0800 0.1527 0.3524 0.5192 0.4049 0.1199 0.1238 1.5384 0.0330 0.5550 0.1154 2.7873 0.0186 0.0677 0.0492 0.1397 0.0929 0.1349 0.0226 0.2095 0.1932 1.0807 0.3451 1.7285 0.43155 Use whatever precision is larger for each data point ------------------------------------------------------------------------ Accuracy of mixing ratios in calibration gas in [%] NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN NaN ------------------------------------------------------------------------ Detection limit (S/N 3/1) in [ppt] per 400 mL air at STP 0.11162 0.53190 0.19529 0.35685 0.18416 0.11912 0.32568 0.47153 0.11040 0.45926 0.30992 3.50523 0.07732 0.74990 0.24115 0.65568 0.25124 0.93355 0.08583 0.39324 0.4981 1.30346 0.625 0.76391 1.86463 Values below detection limit are marked as 0.00 In case no measurements are available, the missing data value is used ------------------------------------------------------------------------ Sample integration time: 147 +- 1 seconds Values of t_sample are the mean of the sampling time interval (integration time) ------------------------------------------------------------------------ Correction of analyte carry-over (memory effect): below measurement precision for all substances, no correction applied Detector non-linearity: below measurement precision for all substances, no correction applied ------------------------------------------------------------------------ 2 TIME C2Cl4 C2H3Cl3 CCl4 CFC11 CFC113 CFC114 CFC115 CFC12 CH2Br2 CH2Cl2 CH3Br CH3Cl CH3I CHBr2Cl CHBr3 CHCl3 H1211 H1301 H2402 HCFC141b HCFC142b HCFC22 HFC125 HFC134a HFC143a [s] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [ppt] [s] [s] 83433.0 0.619 1.327 76.326 226.212 99999.000 15.408 8.555 506.667 1.014 21.129 6.826 561.311 0.286 0.384 0.904 7.188 3.529 3.471 0.000 23.187 22.228 241.501 28.414 102.777 0.000 83788.0 0.481 1.392 76.024 225.769 62.767 15.673 8.959 505.507 0.904 22.370 6.582 558.923 0.171 99999.000 0.514 6.256 3.247 3.052 0.000 23.102 22.283 242.046 28.648 101.451 0.000 84141.0 0.353 1.356 73.622 220.577 61.953 15.371 8.720 499.757 0.691 25.159 7.121 548.433 0.116 0.149 0.202 4.692 3.079 3.466 0.000 22.238 21.690 240.555 28.100 101.011 0.000 84494.0 0.146 1.110 66.386 204.207 58.881 15.037 8.859 480.314 0.484 23.054 6.875 514.823 0.099 99999.000 0.060 3.825 2.807 3.040 0.000 20.604 21.152 233.788 26.776 96.609 0.000 84849.0 0.150 1.263 68.359 207.061 60.397 15.204 8.415 483.290 0.504 23.372 7.037 527.537 0.101 99999.000 0.054 4.701 2.929 3.287 0.000 21.111 21.566 236.174 26.742 96.871 0.000 85203.0 0.107 1.046 62.894 193.890 59.174 14.861 8.196 465.561 0.414 20.223 6.686 494.323 0.099 99999.000 99999.000 3.591 2.688 2.991 0.000 20.228 20.757 229.549 25.361 92.916 0.000 85557.0 0.191 1.114 68.721 207.500 61.949 15.214 8.205 482.085 0.479 22.531 7.078 526.748 0.092 99999.000 0.050 4.232 3.028 2.992 0.000 21.176 21.251 233.369 27.216 96.547 0.000 85911.0 0.222 1.134 69.573 210.091 63.031 15.277 8.426 485.527 0.525 23.090 6.972 530.631 0.086 99999.000 0.071 4.106 3.061 3.164 0.000 21.178 21.212 234.846 26.996 97.510 0.000 86265.0 0.263 1.121 70.322 212.128 63.846 15.343 8.325 490.159 0.566 24.676 7.019 540.251 0.085 99999.000 0.107 4.608 3.101 3.126 0.000 21.483 20.932 237.807 28.235 98.731 0.000 86973.0 0.316 0.959 72.277 216.579 99999.000 15.442 8.776 495.502 0.619 25.568 7.286 551.301 0.078 0.126 0.147 3.971 3.203 3.178 0.000 22.581 21.633 238.923 28.960 100.079 0.000 87327.0 0.406 1.126 74.365 222.861 66.683 15.672 8.530 503.128 0.733 27.234 7.341 567.781 0.090 0.125 0.169 5.575 3.358 3.211 0.000 22.287 22.407 240.334 28.582 102.866 0.000 87681.0 0.522 1.140 76.085 225.527 66.293 15.766 8.247 505.535 0.774 27.287 6.783 590.929 0.086 0.164 0.255 5.857 3.280 3.359 0.000 22.840 22.097 241.847 29.368 102.691 0.000 88036.0 0.507 1.130 75.406 224.759 66.623 15.594 8.458 505.196 0.732 29.684 6.907 588.761 0.081 0.171 0.187 5.631 3.232 3.301 0.000 22.558 22.188 242.310 28.931 102.632 0.000 88390.0 0.246 1.170 69.884 211.239 63.761 15.465 8.543 489.549 0.562 27.108 6.830 546.818 0.075 99999.000 0.074 4.683 3.129 3.227 0.000 21.305 21.330 239.052 27.687 98.294 0.000 88745.0 0.337 1.130 73.310 220.508 65.407 15.478 8.548 501.177 0.630 32.156 6.985 568.046 0.075 99999.000 0.079 5.679 3.227 3.264 0.000 21.878 21.951 241.334 28.789 101.288 0.000 89098.0 0.367 1.230 73.271 223.328 65.829 15.515 8.580 501.459 0.657 32.969 6.915 576.923 0.070 99999.000 0.082 5.619 3.290 3.184 0.000 21.682 22.126 241.918 28.909 102.174 0.000 89452.0 0.227 1.121 68.517 211.049 63.670 15.202 8.789 487.644 0.573 26.386 6.628 548.290 0.108 99999.000 0.056 4.435 2.993 3.095 0.000 21.199 21.508 236.592 27.982 98.219 0.000 89806.0 0.224 1.164 68.136 209.666 63.228 15.368 9.150 486.371 0.556 26.281 6.655 545.252 0.094 99999.000 99999.000 4.459 2.988 3.046 0.000 20.676 21.765 236.634 28.016 98.394 0.000 90512.0 0.149 1.040 63.320 196.504 99999.000 14.917 8.544 467.062 0.454 21.723 6.166 498.065 0.124 99999.000 0.055 3.129 2.703 2.926 0.000 19.918 20.990 230.704 26.504 93.979 0.000 90866.0 0.106 1.213 61.450 191.561 59.255 14.895 8.433 460.940 0.429 19.855 5.982 488.247 0.123 99999.000 99999.000 4.068 2.655 2.840 0.000 19.355 21.238 228.161 25.327 93.014 0.000 91220.0 0.103 1.068 59.757 188.866 58.542 14.895 8.806 457.060 0.407 20.489 6.102 486.393 0.114 99999.000 99999.000 3.624 2.633 2.832 0.000 18.644 21.067 226.116 25.354 92.086 0.000 91573.0 0.102 1.124 63.586 197.979 60.271 15.099 8.469 469.864 0.442 21.758 6.351 503.121 0.127 99999.000 99999.000 3.354 2.788 2.614 0.000 19.319 21.253 232.122 26.525 93.889 0.000 91927.0 0.186 1.124 66.031 205.893 60.951 15.274 8.617 480.279 0.503 25.382 6.662 530.317 0.129 99999.000 99999.000 4.124 3.036 2.842 0.000 19.520 21.402 234.525 26.672 96.583 0.000 92281.0 99999.000 1.047 66.277 206.979 61.848 15.292 8.777 481.020 0.536 26.236 6.705 529.871 0.105 99999.000 99999.000 4.207 2.967 2.784 0.000 19.659 21.413 235.412 28.335 96.719 0.000 92633.0 0.303 1.102 70.368 217.559 62.924 15.434 8.180 493.714 0.652 31.306 7.043 569.810 0.089 99999.000 0.081 4.954 3.171 3.190 0.000 20.235 22.009 240.469 29.496 99.884 0.000 92987.0 0.325 1.150 69.818 217.308 62.520 15.434 8.639 494.309 0.652 31.124 7.109 565.008 0.087 99999.000 0.118 5.474 3.142 3.071 0.000 20.168 21.939 241.743 30.056 99.886 0.000 93340.0 0.155 1.178 64.661 203.018 60.530 15.275 8.307 474.843 0.501 23.525 6.664 512.862 0.099 99999.000 0.061 3.625 2.985 2.940 0.000 19.209 21.520 232.895 26.502 95.832 0.000 94048.0 0.167 1.212 65.073 201.953 99999.000 15.194 8.588 471.692 0.473 22.672 6.606 504.525 0.115 99999.000 0.073 3.779 2.814 3.191 0.000 19.506 21.405 231.722 26.252 96.249 0.000 94401.0 0.131 1.197 64.325 201.335 59.839 15.172 8.651 471.830 0.449 22.686 6.619 507.137 0.106 99999.000 99999.000 4.050 2.716 3.048 0.000 18.993 21.209 232.489 26.311 95.480 0.000 94755.0 0.099 1.156 63.300 199.145 59.498 15.196 8.493 470.852 0.466 21.531 6.482 505.257 0.126 99999.000 0.049 4.285 2.786 3.007 0.000 18.728 21.444 232.302 26.300 95.630 0.000 95108.0 0.126 1.152 59.465 189.735 57.703 14.958 8.431 458.119 0.417 21.346 6.148 479.342 0.112 99999.000 0.042 3.662 2.589 2.840 0.000 18.483 21.015 228.887 25.192 92.214 0.000 95461.0 0.078 0.988 51.098 167.392 53.020 14.460 8.021 429.946 0.280 16.539 5.180 429.922 0.114 99999.000 99999.000 2.778 2.301 2.602 0.000 17.017 20.546 219.190 23.147 88.638 0.000 95815.0 0.080 0.939 52.138 171.492 52.589 14.505 8.147 435.738 0.334 17.132 5.500 439.409 0.139 99999.000 99999.000 2.983 2.375 2.693 0.000 16.898 20.686 222.061 24.068 89.290 0.000 96168.0 0.108 1.102 58.771 191.002 54.713 14.797 8.463 461.841 0.448 20.372 6.160 497.211 0.111 99999.000 99999.000 3.580 2.681 3.038 0.000 17.661 21.463 230.220 26.207 93.572 0.000 96521.0 0.090 1.011 52.758 178.175 50.354 14.735 8.136 443.899 0.352 18.217 5.697 457.774 0.120 99999.000 99999.000 3.024 2.466 2.508 0.000 16.147 21.385 225.416 24.258 90.533 0.000 96875.0 0.084 1.022 56.194 189.641 51.411 14.956 8.612 460.688 0.379 20.057 6.347 492.122 0.123 99999.000 99999.000 3.298 2.661 2.773 0.000 16.508 21.991 228.197 25.418 92.771 0.000 97580.0 0.429 1.125 68.244 223.630 99999.000 15.460 8.516 501.525 0.721 35.232 7.515 578.748 0.108 0.144 0.143 5.301 3.319 3.371 0.000 19.509 22.226 243.173 29.273 102.854 0.000 97934.0 0.195 1.015 61.916 204.655 52.637 15.133 8.635 475.753 0.522 26.976 6.763 523.217 0.102 99999.000 0.068 4.899 2.944 2.909 0.000 17.687 21.708 233.668 27.156 97.205 0.000 98287.0 0.377 1.103 67.807 220.743 51.549 15.287 8.441 497.322 0.705 35.305 7.300 570.353 0.098 0.177 0.130 5.981 3.323 3.194 0.000 18.334 22.218 240.816 28.849 102.143 0.000 98640.0 0.208 1.185 59.827 201.600 47.035 14.905 8.932 472.751 0.499 25.521 6.700 524.385 0.105 99999.000 0.066 4.224 2.894 2.958 0.000 16.113 22.047 230.439 26.802 95.321 0.000 98993.0 0.171 1.098 59.624 203.087 45.032 15.068 8.380 476.950 0.467 25.304 6.888 530.087 0.128 99999.000 99999.000 4.398 2.923 3.089 0.000 15.727 21.742 232.620 27.100 95.548 0.000 99346.0 99999.000 1.288 65.567 223.380 44.743 15.500 8.408 501.027 0.645 34.377 7.610 586.694 0.102 99999.000 0.109 5.954 3.307 3.581 0.000 16.375 22.419 239.593 28.116 102.300 0.000 99700.0 99999.000 1.243 63.794 217.438 40.354 15.385 8.792 492.745 0.572 26.394 7.315 570.405 0.103 99999.000 0.082 4.715 3.178 3.652 0.000 14.898 21.795 235.696 28.065 100.512 0.000 100053.0 0.236 1.247 63.589 217.711 38.420 15.257 8.729 495.498 0.484 99999.000 7.385 569.037 0.088 99999.000 0.062 99999.000 3.165 3.266 0.000 14.427 22.114 237.171 27.890 99.144 0.000 100407.0 0.290 1.026 63.794 222.235 35.688 15.509 8.639 500.072 0.480 99999.000 7.635 576.706 0.092 99999.000 0.074 99999.000 3.166 3.498 0.000 13.614 22.221 241.423 28.810 102.347 0.000 101112.0 0.336 0.889 65.522 223.418 99999.000 15.448 8.779 502.604 0.555 30.515 7.489 583.140 0.094 99999.000 0.109 5.071 3.210 3.504 0.000 14.885 22.056 242.214 29.685 102.305 0.000 101465.0 0.286 0.902 60.877 219.951 29.570 15.360 8.739 497.786 0.341 99999.000 7.320 575.353 0.074 99999.000 0.101 99999.000 3.178 3.525 0.000 11.420 22.169 239.593 28.629 102.079 0.000 101817.0 0.224 0.958 59.242 218.740 26.671 15.550 8.764 497.593 0.374 99999.000 7.234 574.705 0.088 99999.000 99999.000 99999.000 3.181 3.299 0.000 10.717 22.082 240.160 28.446 100.775 0.000 102171.0 0.215 0.986 58.424 218.516 25.263 15.432 8.925 495.665 0.377 99999.000 7.180 579.509 0.089 99999.000 0.066 99999.000 3.168 3.338 0.000 9.802 21.898 239.772 29.466 100.393 0.000 102524.0 0.183 1.162 57.528 217.008 23.021 15.560 8.940 497.089 0.253 99999.000 7.262 586.388 0.116 99999.000 0.065 99999.000 3.068 3.284 0.000 9.237 22.163 239.639 28.645 99.633 0.000 102877.0 0.220 0.998 57.609 217.677 22.373 15.513 8.651 495.311 0.241 99999.000 7.174 573.398 0.100 99999.000 0.057 99999.000 3.107 3.124 0.000 8.610 22.101 239.150 28.962 100.230 0.000 103231.0 0.199 1.004 57.365 216.087 20.257 15.551 8.732 495.769 0.195 18.230 7.337 574.433 0.087 99999.000 0.051 99999.000 3.021 2.963 0.000 8.162 21.975 240.895 28.647 100.642 0.000 103585.0 0.169 1.077 57.366 216.827 19.074 15.504 8.906 492.765 0.160 16.762 7.215 574.746 0.085 99999.000 0.045 99999.000 3.045 3.072 99999.000 7.859 22.470 242.245 29.345 99.485 0.000 103937.0 0.164 1.152 56.292 216.289 17.769 15.474 8.838 494.065 0.135 99999.000 7.233 571.685 0.093 99999.000 0.051 99999.000 3.031 2.980 99999.000 7.303 22.316 239.588 28.420 100.079 0.000 104644.0 0.283 1.079 58.330 223.303 99999.000 15.813 8.317 501.506 0.221 99999.000 7.386 585.684 0.084 99999.000 0.125 99999.000 3.148 3.138 0.000 8.168 22.519 242.805 29.313 102.286 0.000 104996.0 0.222 1.097 58.650 225.117 16.066 15.717 8.477 505.589 99999.000 18.759 7.315 594.447 99999.000 99999.000 0.126 99999.000 3.222 3.080 99999.000 6.810 22.622 244.552 29.250 103.368 0.000 105350.0 0.195 99999.000 57.536 223.635 15.140 15.548 8.397 503.516 99999.000 99999.000 7.300 591.297 0.091 99999.000 0.105 99999.000 3.246 2.904 99999.000 6.445 22.462 245.863 29.102 103.363 0.000 105702.0 0.188 1.320 61.158 224.537 14.378 15.776 8.453 503.655 99999.000 15.083 7.157 588.558 99999.000 99999.000 0.084 99999.000 3.290 2.939 99999.000 6.069 22.372 245.688 29.408 102.849 0.000 106056.0 0.149 1.333 55.739 225.662 13.399 15.582 7.793 505.085 99999.000 99999.000 7.123 589.620 99999.000 99999.000 0.117 99999.000 3.305 2.951 99999.000 5.679 22.711 246.965 28.741 104.762 0.000 106409.0 0.188 1.245 99999.000 226.733 12.956 15.780 8.133 505.141 99999.000 99999.000 7.275 593.842 99999.000 0.154 0.125 99999.000 3.302 3.419 99999.000 5.520 22.278 245.979 29.726 104.297 0.000 106763.0 0.117 1.272 99999.000 224.716 12.172 15.617 8.655 503.653 99999.000 16.176 7.151 593.225 99999.000 99999.000 0.096 99999.000 3.196 3.182 99999.000 5.430 22.200 246.016 30.211 102.961 0.000 107115.0 99999.000 1.351 99999.000 225.112 11.501 15.722 9.181 503.064 99999.000 99999.000 7.463 600.520 99999.000 99999.000 0.082 99999.000 3.329 3.322 99999.000 4.977 22.240 244.581 29.281 103.437 0.000 107468.0 99999.000 99999.000 99999.000 225.611 11.163 15.632 8.617 503.215 99999.000 99999.000 7.043 595.237 99999.000 99999.000 0.070 99999.000 3.294 3.418 99999.000 4.823 22.159 247.221 29.706 103.198 0.000 108173.0 0.093 99999.000 99999.000 226.752 99999.000 15.674 8.923 504.236 99999.000 99999.000 7.302 592.397 99999.000 99999.000 0.088 99999.000 3.304 3.301 99999.000 5.129 22.348 245.197 29.296 104.387 0.000 108526.0 0.057 1.009 99999.000 225.168 10.373 15.806 8.700 503.778 99999.000 99999.000 7.419 590.016 99999.000 99999.000 0.061 99999.000 3.287 3.586 99999.000 4.490 22.219 246.837 29.773 103.104 0.000 108879.0 99999.000 0.966 99999.000 223.754 9.902 15.722 8.373 501.290 99999.000 99999.000 7.461 588.561 99999.000 99999.000 0.056 99999.000 3.288 3.372 99999.000 4.316 22.461 245.905 28.819 102.561 0.000 109232.0 99999.000 0.806 99999.000 226.587 9.804 15.797 9.009 507.094 99999.000 99999.000 7.633 594.179 99999.000 99999.000 0.069 99999.000 3.296 3.655 99999.000 4.332 22.499 245.154 30.042 103.649 0.000 109585.0 99999.000 99999.000 99999.000 224.155 9.544 15.841 8.682 503.945 99999.000 99999.000 7.773 601.045 99999.000 99999.000 0.072 99999.000 3.371 3.363 99999.000 99999.000 22.214 246.221 30.527 102.968 0.000 110996.0 0.625 1.261 76.315 225.483 99999.000 15.687 8.738 506.644 1.021 22.681 8.687 626.326 0.270 0.459 0.852 7.215 3.276 3.365 0.000 23.154 22.553 237.818 27.894 99.150 0.000 111350.0 0.555 1.380 77.744 227.928 57.637 15.773 8.908 507.956 1.029 20.555 6.448 550.211 0.215 0.367 0.929 6.760 3.340 3.626 0.000 23.835 22.364 240.334 28.951 100.434 0.000 111705.0 0.572 1.251 78.180 227.295 60.009 15.726 8.931 508.199 1.032 20.258 6.155 544.494 0.209 0.340 0.960 6.877 3.132 3.285 0.000 23.658 22.002 239.870 28.024 101.820 0.000 112059.0 0.555 1.271 77.260 225.354 62.169 15.556 9.242 504.908 1.076 20.049 6.805 542.871 0.261 0.486 1.652 7.717 3.184 3.378 0.000 23.597 22.748 238.602 27.851 99.995 0.000 112413.0 0.533 1.238 76.631 225.010 65.056 15.418 8.976 505.790 1.019 19.927 6.070 538.396 0.264 0.414 1.325 7.252 3.256 3.326 0.000 23.331 22.698 238.697 28.272 99.039 0.000 112768.0 0.516 1.302 76.754 225.604 67.698 15.296 8.959 505.335 1.052 19.670 6.065 541.208 0.235 0.400 1.391 7.758 3.217 3.528 0.000 23.578 22.688 236.412 28.322 99.331 0.000